Understanding the Low-Frequency Quasilocalized Modes in Disordered Colloidal Systems

Peng Tan, Ning Xu, Andrew B. Schofield, and Lei Xu
Phys. Rev. Lett. 108, 095501 – Published 27 February 2012

Abstract

In disordered colloidal systems, we experimentally measure the normal modes with the covariance matrix method and clarify the origin of low-frequency quasilocalization at the single-particle level. We observe important features from both jamming and glass simulations: There is a plateau in the density of states [D(ω)] which is suppressed upon compression, as predicted by jamming; within the same systems, we also find that the low-frequency quasilocalization originates from the large vibrations of defective structures coupled with transverse excitations, consistent with a recent glass simulation. The coexistence of these features demonstrates an experimental link between jamming and glass. Extensive simulations further show that such a structural origin of quasilocalization is universally valid for various temperatures and volume fractions.

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  • Received 7 November 2011

DOI:https://doi.org/10.1103/PhysRevLett.108.095501

© 2012 American Physical Society

Authors & Affiliations

Peng Tan1, Ning Xu2, Andrew B. Schofield3, and Lei Xu1

  • 1Department of Physics, The Chinese University of Hong Kong, Hong Kong, People’s Republic of China
  • 2Hefei National Laboratory for Physical Sciences at the Miscroscale, CAS Key Laboratory of Soft Matter Chemistry, and Department of Physics, University of Science and Technology of China, Hefei 230026, People’s Republic of China
  • 3The School of Physics, University of Edinburgh, Edinburgh EH9 3 JZ, United Kingdom

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Issue

Vol. 108, Iss. 9 — 2 March 2012

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